Mechanically controlled FRET to achieve high-contrast fluorescence switching

Shenzhong Mo; Lina Tan; Bing Fang; Zhen Wu; Zhiqiang Su; Yantu Zhang; Meizhen Yin

doi:10.1007/s11426-018-9303-9

SCIENCE CHINA Chemistry

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SCIENCE CHINA Chemistry, Volume 61, Issue 12: 1587-1593(2018) https://doi.org/10.1007/s11426-018-9303-9

Mechanically controlled FRET to achieve high-contrast fluorescence switching

Shenzhong Mo¹, Lina Tan¹, Bing Fang¹, Zhen Wu¹, Zhiqiang Su¹, Yantu Zhang^2,*, Meizhen Yin^1,*

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ReceivedMay 17, 2018
AcceptedJun 5, 2018
PublishedAug 30, 2018

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Abstract

Organic luminescent materials with the ability to reversibly switch the luminescence when subjected to external stimuli have attracted considerable interest in recent years. However, luminescent materials with mechanochromic and photochromic dual-responsive properties are rarely reported. Hererin, we designed and synthesized a molecule P1 with dipeptide as a spacer to link rhodamine B and spiropyran moieties. P1 exhibited efficient photochromic properties both in solution and solid state. High-contrast independent fluorescence switch was also realized under the stimulus of external force. Moreover, two-step ring opening reaction and subsequent fluorescence resonance energy transfer process between the donor-acceptor pairs within one single molecule achieved successive color switch by mechanical control. Therefore, this behavior of P1 made it a promising candidate for high-contrast and sensitive optical recording and mechanical sensing system.

Funded by

the National Natural Science Foundation of China(21774007,21574009,51521062)

the Natural Science Foundation of Shaanxi Province

China(2016ZDJC19)

Yan’an Science & Technology Innovation Team(2015CHTD-04)

Acknowledgment

This work was supported by the National Natural Science Foundation of China (21774007, 21574009, 51521062), the Natural Science Foundation of Shaanxi Province, China (2016ZDJC19) and Yan’an Science & Technology Innovation Team (2015CHTD-04).

Interest statement

The authors declare that they have no conflict of interest.

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Supporting Information

The supporting information is available online at http://chem.scichina.com and http://link.springer.com/journal/11426. The supporting materials are published as submitted, without typesetting or editing. The responsibility for scientific accuracy and content remains entirely with the authors.

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Mechanically controlled FRET to achieve high-contrast fluorescence switching

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